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NO reduction by propene or CO over alkali-promoted Pd/YSZ catalysts

Konsolakis Michail, Gentekakis Ioannis

Πλήρης Εγγραφή


URI: http://purl.tuc.gr/dl/dias/56C8375A-728F-4201-A7CB-D05F092DE726
Έτος 2007
Τύπος Δημοσίευση σε Περιοδικό με Κριτές
Άδεια Χρήσης
Λεπτομέρειες
Βιβλιογραφική Αναφορά M. Konsolakis and I. V. Yentekakis, "NO reduction by propene or CO over alkali-promoted Pd/YSZ catalysts", J. Hazardous Mater., vol. 149, no. 3, pp. 619-624, Nov. 2007. doi:10.1016/j.jhazmat.2007.06.085 https://doi.org/10.1016/j.jhazmat.2007.06.085
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Περίληψη

The catalytic activity and selectivity of Pd dispersed on 8 mol% yttria stabilized zirconia (YSZ) support for the reduction of NO by propene or CO is strongly promoted by alkalis in a wide temperature range 200–500 °C. Rate increases by up to one order of magnitude are achievable, accompanied with significant improvement in N2-selectivity for the alkali promoted catalysts. The promoting effect of alkalis on both the activity and selectivity can be understood in terms of the effect of alkali promoter on the relative adsorption strengths of reactant species. These achievements could be very useful for the formulation of modern lower cost automotive catalytic converters, capable of controlling automotive emissions more efficiently.

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